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JAEA Reports

Development of rapid and sensitive radionuclide analysis method by simultaneous analysis of $$beta$$, $$gamma$$, and X-rays (Contract research); FY2022 Nuclear Energy Science & Technology and Human Resource Development Project

Collaborative Laboratories for Advanced Decommissioning Science; Japan Chemical Analysis Center*

JAEA-Review 2023-022, 93 Pages, 2023/12

JAEA-Review-2023-022.pdf:4.7MB

The Collaborative Laboratories for Advanced Decommissioning Science (CLADS), Japan Atomic Energy Agency (JAEA), had been conducting the Nuclear Energy Science & Technology and Human Resource Development Project (hereafter referred to "the Project") in FY2022. The Project aims to contribute to solving problems in the nuclear energy field represented by the decommissioning of the Fukushima Daiichi Nuclear Power Station, Tokyo Electric Power Company Holdings, Inc. (TEPCO). For this purpose, intelligence was collected from all over the world, and basic research and human resource development were promoted by closely integrating/collaborating knowledge and experiences in various fields beyond the barrier of conventional organizations and research fields. The sponsor of the Project was moved from the Ministry of Education, Culture, Sports, Science and Technology to JAEA since the newly adopted proposals in FY2018. On this occasion, JAEA constructed a new research system where JAEA-academia collaboration is reinforced and medium-to-long term research/development and human resource development contributing to the decommissioning are stably and consecutively implemented. Among the adopted proposals in FY2020, this report summarizes the research results of the "Development of rapid and sensitive radionuclide analysis method by simultaneous analysis of $$beta$$, $$gamma$$, and X-rays" conducted from FY2020 to FY2022. The present study aims to enable rapid analysis of radionuclides in fuel debris and waste, we have established the latest measurement system, such as the multiple $$gamma$$-ray detection methods, and the Spectral Determination Method (hereinafter referred to as "SDM") was developed. In the research in 2022, we developed a code that handles measurement data of LSC, singles Ge, and 2D spectra (multiple $$gamma$$). In addition, to develop an integrated database, spectral data of 40 nuclides were obtained by actual measurements and simulation calculations.

JAEA Reports

Development of rapid and sensitive radionuclide analysis method by simultaneous analysis of $$beta$$, $$gamma$$, and X-rays (Contract research); FY2021 Nuclear Energy Science & Technology and Human Resource Development Project

Collaborative Laboratories for Advanced Decommissioning Science; Japan Chemical Analysis Center*

JAEA-Review 2022-037, 118 Pages, 2023/01

JAEA-Review-2022-037.pdf:6.92MB

The Collaborative Laboratories for Advanced Decommissioning Science (CLADS), Japan Atomic Energy Agency (JAEA), had been conducting the Nuclear Energy Science & Technology and Human Resource Development Project (hereafter referred to "the Project") in FY2021. The Project aims to contribute to solving problems in the nuclear energy field represented by the decommissioning of the Fukushima Daiichi Nuclear Power Station, Tokyo Electric Power Company Holdings, Inc. (TEPCO). For this purpose, intelligence was collected from all over the world, and basic research and human resource development were promoted by closely integrating/collaborating knowledge and experiences in various fields beyond the barrier of conventional organizations and research fields. The sponsor of the Project was moved from the Ministry of Education, Culture, Sports, Science and Technology to JAEA since the newly adopted proposals in FY2018. On this occasion, JAEA constructed a new research system where JAEA-academia collaboration is reinforced and medium-to-long term research/development and human resource development contributing to the decommissioning are stably and consecutively implemented. Among the adopted proposals in FY2020, this report summarizes the research results of the "Development of rapid and sensitive radionuclide analysis method by simultaneous analysis of $$beta$$, $$gamma$$, and X-rays" conducted in FY2021. The present study aims to enable rapid analysis of radionuclides in fuel debris and waste, we have established the latest measurement system, such as the multiple $$gamma$$-ray detection methods, and the Spectral Determination Method (hereafter referred to "SDM") was developed. In the study, the $$gamma$$-ray measuring device was installed, and the measurement system consisting of the Ge detector, CeBr$$_{3}$$ detector, and NaI detector was completed in FY2021. In the SDM development, standard spectra of $$gamma$$-ray singles, multiple $$gamma$$-ray measurements, …

JAEA Reports

Development of rapid and sensitive radionuclide analysis method by simultaneous analysis of $$beta$$, $$gamma$$, and X-rays (Contract research); FY2020 Nuclear Energy Science & Technology and Human Resource Development Project

Collaborative Laboratories for Advanced Decommissioning Science; Japan Chemical Analysis Center*

JAEA-Review 2021-060, 105 Pages, 2022/03

JAEA-Review-2021-060.pdf:4.59MB

The Collaborative Laboratories for Advanced Decommissioning Science (CLADS), Japan Atomic Energy Agency (JAEA), had been conducting the Nuclear Energy Science & Technology and Human Resource Development Project (hereafter referred to "the Project") in FY2020. The Project aims to contribute to solving problems in the nuclear energy field represented by the decommissioning of the Fukushima Daiichi Nuclear Power Station, Tokyo Electric Power Company Holdings, Inc. (TEPCO). For this purpose, intelligence was collected from all over the world, and basic research and human resource development were promoted by closely integrating/collaborating knowledge and experiences in various fields beyond the barrier of conventional organizations and research fields. The sponsor of the Project was moved from the Ministry of Education, Culture, Sports, Science and Technology to JAEA since the newly adopted proposals in FY2018. On this occasion, JAEA constructed a new research system where JAEA-academia collaboration is reinforced and medium-to-long term research/development and human resource development contributing to the decommissioning are stably and consecutively implemented. Among the adopted proposals in FY2020, this report summarizes the research results of the "Development of rapid and sensitive radionuclide analysis method by simultaneous analysis of $$beta$$, $$gamma$$, and X-rays" conducted in FY2020. The present study aims to enable rapid analysis of radionuclides in fuel debris and waste, and develops the measurement system such as multiple $$gamma$$-ray detection method. We develop a spectral determination method (SDM method) for integrated analysis by constructing a spectral database for nuclides including $$beta$$-rays and X-rays by measurement using this system and radiation simulation calculation. This method enables simultaneous quantification of multiple nuclides and reduces the chemical separation process.

Journal Articles

Present status and future perspective of research and development on partitioning and transmutation technology at JAERI

Oigawa, Hiroyuki; Minato, Kazuo; Kimura, Takaumi; Morita, Yasuji; Arai, Yasuo; Nakayama, Shinichi; Nishihara, Kenji

Proceedings of International Conference on Nuclear Energy System for Future Generation and Global Sustainability (GLOBAL 2005) (CD-ROM), 6 Pages, 2005/10

JAERI is engaging in the R&D on the Double-strata Fuel Cycle concept in accordance with the results of the check and review on the Partitioning and Transmutation (PT) technology made by the Atomic Energy Commission of Japan in 2000. As for the partitioning process, after the establishment of the "4-group Partitioning Process Concept", an innovative concept called ARTIST is also being studied. As for the fuel technology, minor actinide nitrides such as NpN and AmN were synthesized and their material properties have been measured. To reprocess the irradiated fuel, the pyrochemical process has been studied. The R&D of the accelerator-driven transmutation system are in progress for an accelerator, lead-bismuth, and a subcritical reactor. In addition, JAERI has started the high-intensity proton accelerator project (J-PARC), which includes the Transmutation Experimental Facility (TEF) as the Phase-II. The impact of PT technology on the backend of the nuclear energy utilization is also being discussed.

Journal Articles

Long-lived nuclide separation for advancing back-end fuel cycle process

Uchiyama, Gunzo; Mineo, Hideaki; Asakura, Toshihide; Hotoku, Shinobu; Iizuka, Masaru*; Fujisaki, Susumu; Isogai, Hikaru; Ito, Yoshinori*; Sato, Makoto; Hosoya, Noriaki

Journal of Nuclear Science and Technology, 39(Suppl.3), p.925 - 928, 2002/11

no abstracts in English

Journal Articles

Development of an advanced reprocessing process of spent nuclear fuel

Uchiyama, Gunzo; Mineo, Hideaki; Asakura, Toshihide; Hotoku, Shinobu

Nihon Kikai Gakkai Dai-8-Kai Doryoku, Enerugi Gijutsu Shimpojiumu Koen Rombunshu, p.483 - 488, 2002/00

no abstracts in English

Journal Articles

Advanced technologies for long-lived nuclides separation in reprocessing

Uchiyama, Gunzo; Mineo, Hideaki; Asakura, Toshihide; Hotoku, Shinobu

Proceedings of International Conference on Back-End of the Fuel Cycle: From Research to Solutions (GLOBAL 2001) (CD-ROM), 8 Pages, 2001/09

no abstracts in English

Journal Articles

R&D of partitioning and transmutation; Aiming at improvement of HLW disposal

Mukaiyama, Takehiko

Genshiryoku eye, 44(2), p.15 - 19, 1998/02

no abstracts in English

Journal Articles

Extraction behaviors of uranium, plutonium, neptunium and technetium in PARC process

Uchiyama, Gunzo; Asakura, Toshihide; Hotoku, Shinobu; Fujine, Sachio

Proc. of 5th Int. Nucl. Conf. on Recycling, Conditioning and Disposal (RECOD '98), 1, p.393 - 400, 1998/00

no abstracts in English

Journal Articles

Analysis of nuclear fuels, reactor and environmental materials

Watanabe, Kazuo;

Bunseki, 1993(11), p.883 - 889, 1993/00

no abstracts in English

Journal Articles

Long-lived radionuclide transport; An In-situ field column study

D.R.Champ*; J.O.Jirovec*; J.L.Young*; Kumata, Masahiro

Transport and Mass Exchange Processes in Sand and Gravel Aquifers; Field and Modelling Studies,Vol. 2, p.725 - 736, 1991/00

no abstracts in English

11 (Records 1-11 displayed on this page)
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